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aktuelle Publikationen 2019


Comparative Microstructural Analysis of Non-graphitic Carbons by Wide-angle X-ray and Neutron Scattering
T. Pfaff · F.  Badaczewski · M. O. Loeh · A. Franz · J.-U. Hoffmann · M. Reehuis · W. G. Zeier · B. M. Smarsly
The Journal of Physical Chemistry C 2019 (accepted), DOI: 10.1021/acs.jpcc.9b03590


Making It Clear: Exploring Crystal Structures by Constructing and Comparing See-Through Models
S. Lenzer ·  B. M. Smarsly · N. Graulich
Journal of Chemical Education 2019, 96, 1630-1639, DOI: 10.1021/acs.jchemed.9b00119


Atomic Layer Deposition of Titania in Ordered Mesoporous Cerium Zirconium Oxide Thin Films: A Case Study
P. Cop · M. Göttlicher · J. Schörmann · C. Boissiere · A. Beyer · C. Becker · K. Volz · H. Over · B. M. Smarsly
The Journal of Physical Chemistry C 2019, 123, 12851-12861, DOI: 10.1021/acs.jpcc.9b02069


Independent Tailoring of Macropore and Mesopore Space in TiO2 Monoliths
G. Beck · M. Sieland · J. F. Beleites · R. Marschall · B. M. Smarsly
Inorganic Chemistry 2019, 58, 2599-2609, DOI: 10.1021/acs.inorgchem.8b03203


Electrospun CuO Nanofibre Assemblies for H2S Sensing
C. Seitz · S. Werner · R. Marschall · B. M. Smarsly
Zeitschrift für Physikalische Chemie 2019, 233, 105-116 DOI: 10.1515/zpch-2017-1097



aktuelle Publikationen 2018


Structural characterization and magnetic properties determination of nanocrystalline Ba3Fe2WO9 and Sr3Fe2WO9 perovskites prepared by the modified aqueous sol-gel route
J. Bijelić · A. Stanković · B. Matasović · B. Marković · M. Bijelić · Ž. Skoko · J. Popović · G. Štefanić · Z. Jagličić · S. Zellmer · T. Preller · G. Garnweitner · T. Đorđević · P. Cop · B. M. Smarsly · I. Djerdj
CrystEngComm 2019, 21, 218-227, DOI: 10.1039/C8CE01483C


Peering into the structural evolution of glass-like carbons derived from phenolic resin by combining small-angle neutron scattering with an advanced evaluation method for wide-angle X-ray scattering
F. Badaczewski · M. O. Loeh · T. Pfaff · S. Dobrotka · D. Wallacher · D. Clemens · J. Metz · B. M. Smarsly
Carbon 2019, 141, 169-181, DOI: 10.1016/j.carbon.2018.09.025


Mechanochemical synthesis of porous carbon at room temperature with a highly ordered sp2 microstructure
M. E. Casco · F. Badaczewski · S. Grätz · A. Tolosa · V. Presser · B. M. Smarsly · L. Borchardt
Carbon 2018, 139, 325-333, DOI: 10.1016/j.carbon.2018.06.068


Hydrophilic Ionic Liquid Mixtures of Weakly and Strongly Coordinating Anions with and without Water
R. Macchieraldo · L. Essert · R. Elfgen · P. Vöpel · B. M. Smarsly · B. Kirchner
ACS Omega 2018, 3, 8567-8582, DOI: 10.1021/acsomega.8b00995


The Critical Role of the Crystallite Size in Nanostructured Li4Ti5O12 Anodes for Lithium Ion Batteries
J. Yue · F. Badaczewski · P. Voepel · T. Leichtweiß · D. Mollenhauer · W. Zeier · B. M. Smarsly
ACS Applied Materials and Interfaces 2018, 10, 22580-22590, DOI: 10.1021/acsami.8b05057


In-plane stress development in mesoporous thin films
P. Cop · S. Kitano · K. Niinuma · B. M. Smarsly · H. Kozuka
Nanoscale 2018, 10, 7002-7015, DOI: 10.1039/c8nr00793d
Koorperation mit der AG Kozuka (Kansai-University Osaka)


Nitrogen-containing novolac-derived carbon beadsas electrode material for supercapacitors
B. Krüner · A. Schreiber · A. Tolosoa · A. Quade · F. Badaczewski · T. Pfaff · B. M. Smarsly · V. Presser
Carbon 2018, 132, 220-231, DOI: 10.1016/j.carbon.2018.02.029


CarbX: a program for the evaluation of wide-angle X-ray scattering data of non-graphitic carbons
T. Pfaff · M. Simmermacher · B. M. Smarsly
Journal of Applied Crystallography 2018, 51, 219-229, DOI: 10.1107/S1600576718000195


Mesoporous Poly(divinylbenzene) Fibers Based On Crosslinked Nanoparticles
J. Migenda · S. Werner · R. Ellinghaus · B. M. Smarsly
Macromolecular Chemistry and Physics 2018, 219, 1700471 DOI: 10.1002/macp.201700471


Electrospinning of CeO2 nanoparticle dispersions into mesoporous fibers: on the interplay of stability and activity in the HCl oxidation reaction
M. Möller · N. Tarabanko · C. Wessel · R. Ellinghaus · H. Over · B. M. Smarsly
RSC Advances 2018, 8, 132-144 DOI: 10.1039/C7RA03020G


The stabilizing effect of water and high reaction temperatures on the CeO2-catalyst in the harsh HCl oxidation reaction
C. Li · F. Hess · I. Djerdj · G. Chai · Y. Sun · Y. Guo · B. M. Smarsly · H. Over
Journal of Catalysis 2018, 357, 257-262, DOI: 10.1016/j.jcat.2017.11.019
Koorperation mit der AG Over


Hard-templating of carbon using porous SiO2 monoliths revisited - Quantitative impact of spatial confinement on the microstructure evolution
M. O. Loeh · F. Badaczewski · M. von der Lehr · R. Ellinghaus · S. Dobrotka · J. Metz · B. M. Smarsly
Carbon 2018, 129, 552-563, DOI: 10.1016/j.carbon.2017.12.044



aktuelle Publikationen 2017


Peering into the Mechanism of Low-Temperature Synthesis of Bronze-type TiO2 in Ionic Liquids
P. Vöpel · C. Seitz · J. M. Waack · S. Zahn · T. Leichtweiß · A. Zaichenko · D. Mollenhauer · H. Amenitsch · M. Voggenreiter · S. Polarz · B. M. Smarsly
Crystal Growth and Design 2017, 17, 5586-5601, DOI: 10.1021/acs.cgd.7b01231


On the underestimated impact of the gelation temperature on macro- and mesoporosity in monolithic silica
R. Meinusch · R. Ellinghaus · K. Hormann · U. Tallarek · B. M. Smarsly
Physical Chemistry Chemical Physics 2017, 19, 14821-14834, DOI: 10.1039/C7CP01846K


Sustainable and surfactant-free high-throughput synthesis of highly dispersible zirconia nanocrystals
C. Suchomski · D. J. Weber · P. Dolcet · A. Hofmann · P. Vopel · J. Yue · M. Einert · M. Möller · S. Werner · S. Gross · I. Derdj · T. Brezesinski · B. M. Smarsly
Journal of Materials Chemistry A - Materials for energy and sustainability 2017, 5, 16296-16306, DOI: 10.1039/C7TA02316B, Supp. Inf.


Mesopore etching under supercritical conditions - A shortcut to hierarchically porous silica monoliths
M. von der Lehr · K. Hormann · A. Höltzel · L. S. White · A. E. Reising · M. F. Bertino · B. M. Smarsly · U. Tallarek
Microporous and Mesoporous Materials 2017, 243, 247-253, DOI: 10.1016/j.micromeso.2017.02.036


Mesoporous niobium-doped titanium dioxide films from the assembly of crystalline nanoparticles: study on the relationship between the band structure, conductivity and charge storage mechanism
J. Yue · C. Suchomski · P. Vöpel · R. Ellinghaus · M. Rohnke · T Leichtweiss · M. T. Elm · B. M. Smarsly
Journal of Materials Chemistry A - Materials for energy and sustainability 2017, 5, 1978-1988, DOI: 10.1039/c6ta06840e


Low Temperature Reaction of Molecular Zinc Oxide Precursors in Ionic Liquids Leading to Ionogel Nanoparticles with Shape Anisotropy
M.Voggenreiter · P. Vöpel · B. M. Smarsly · S. Polarz
Journal of Inorganic and General Chemistry 2017, 643, 93-100, DOI: 10.1002/zaac.201600341


Synthesis of Titanium Oxide Nanostructures in Ionic Liquids
P. Vöpel · B. M. Smarsly
Journal of Inorganic and General Chemistry 2017, 643, 3-13, DOI: 10.1002/zaac.201600394



aktuelle Publikationen 2016


Highly Active Binder-Free Catalytic Coatings for Heterogeneous Catalysis and Electrocatalysis: Pd on Mesoporous Carbon and Its Application in Butadiene Hydrogenation and Hydrogen Evolution
D. Bernsmeier · L. Chuenchom · B. Paul · S. Rümmler · B. M. Smarsly · R. Kraehnert
ACS Catalysis 2016, 6 (12), 8255-8263, DOI: 10.1021/acscatal.6b02240


Hollow a-Fe2O3 Nanofibres for Solar Water Oxidation: Improving the Photoelectrochemical Performance by Formation of a-Fe2O3/ITO-Composite Photoanodes
M. Einert · R. Ostermann · T. Weller · S. Zellmer · G. Garnweitner · B. M. Smarsly · R. Marschall
Journal of Materials Chemistry A - Materials for energy and sustainability 2016, 4, 18444-18456, DOI: 10.1039/C6TA06979G


Analysis of thermally induced changes in the structure of coal tar pitches by an advanced evaluation method of X-ray scattering data
M. O. Loeh · F. Badaczewski · K. Faber · S. Hintner · M.F. Bertino· P. Mueller· J. Metz · B. M. Smarsly
Carbon 2016, 109, 823-835, DOI: 10.1016/j.carbon.2016.08.031


Synthesis and full characterization of the phase-pure pyrochlore Ce2Zr2O7 and the κ-Ce2Zr2O8 phases
S. Urban · P. Dolcet · M. Möller · L. Chen · P. J. Klar · I. Djerdj · S. Gross · B. M. Smarsly · H. Over
Applied Catalysis B: Environmental 2016, 197, 23-34, DOI:0.1016/j.apcatb.2016.03.049


Proton Conduction in Sulfonated Organic–Inorganic Hybrid Monoliths with Hierarchical Pore Structure
M. von der Lehr · C. F. Seidler · D. H. Taffa · M. Wark · B. M. Smarsly · R. Marschall
ACS Applied Materials and Interfaces 2016, 8 (38), 25476-25488, DOI:10.1021/acsami.6b08477


Hierarchically porous monolithic silica with varying porosity using bis(trimethoxysilyl)arenes as precursors
M. von der Lehr · R. Ellinghaus · B. M. Smarsly
New Journal of Chemistry 2016, 40, 4455-4463, DOI:10.1039/C6NJ00758A


Aqueous Sol–Gel Route toward Selected Quaternary Metal Oxides with Single and Double Perovskite-Type Structure Containing Tellurium
Igor Djerdj · J. Popovic · S. Mal · T. Weller · M. Nuskol · Z. Jaglicic · Z. Skoko · D. Pajic· C. Suchomski · P. Vöpel · R. Marschall · B. Kozlevcar · B. M. Smarsly
Crystal Growth Design 2016, 16 (5), 2535-2541, DOI:10.1021/acs.cgd.5b01558


Engineering of oxoclusters-reinforced polymeric materials with application as heterogeneous oxydesulfurization catalysts
M. Vigolo · S. Borsacchi · A. Sorarù · M. Geppi · B. M. Smarsly · P. Dolcet · S. Rizzato · M. Carraro · S. Gross
Applied Catalysis B: Environmental 2016, 182, 636-644, DOI:10.1016/j.apcatb.2015.10.008


In-depth mesocrystal formation analysis of microwave-assisted synthesis of LiMnPO4 nanostructures in organic solution
P. Vöpel · C. Suchomski · A. Hofmann · S. Gross · P. Dolcet · B. M. Smarsly
CrystEngComm 2016, 18, 316-327, DOI: 10.1039/C5CE01946J



aktuelle Publikationen 2014/15


Nitrogen-Doped Carbon Electrodes: Influence of Microstructure and Nitrogen Configuration on the Electrical Conductivity of Carbonized Polyacrylonitrile and Poly(ionic liquid) Blends
Marcus Einert · Claas Wessel · Felix Badaczewski · Thomas Leichtweiß · Christine Eufinger · Jürgen Janek · Jiayin Yuan · Markus Antonietti · Bernd M. Smarsly
Macromolecular Chemistry and Physics 10/2015; 216(19):1909-1909. DOI: 10.1002/macp.201500169 (Paper), 10.1002/macp.201570059 (Front Cover)

Polymer Templated Mesoporous Li4Ti5O12 as a High-Rate and Long-Life Anode Material for Rechargeable Li-Ion Batteries
Junpei Yue · Christian Suchomski · Bernd M. Smarsly · Torsten Brezesinski
08/2015; DOI: 10.1002/cnma.201500078

Mechanisms of Charge Storage in Nanoparticulate TiO2 and Li4Ti5O12 Anodes: New Insights from Scan rate-dependent Cyclic Voltammetry
Martin Opitz · Junpei Yue · Jens Wallauer · Bernd Smarsly · Bernhard Roling
Electrochimica Acta 06/2015; 168:125-132. DOI: 10.1016/j.electacta.2015.03.186

Ionic Liquid- and Surfactant-Controlled Crystallization of WO3 films
Helena Kaper · Igor Djerdj · Silvia Gross · Heinz Amenitsch · Markus Antonietti · Bernd M Smarsly
Physical Chemistry Chemical Physics 05/2015; 17(27). DOI: 10.1039/C5CP01869B

Elucidating the Sorption Mechanism of Dibromomethane in Disordered Mesoporous Silica Adsorbents
Daniela Stoeckel · Dirk Wallacher · Gerald A. Zickler · Matthias Thommes · Bernd M Smarsly
Langmuir 05/2015; 31(23). DOI: 10.1021/acs.langmuir.5b00705

Electrospun ceria-based nanofibers for the facile assessment of catalyst morphological stability under harsh HCl oxidation reaction conditions
Maren Möller · Herbert Over · Bernd Smarsly · Nikolay Tarabanko · Sven Urban
Catalysis Today 04/2015; 253. DOI: 10.1016/j.cattod.2015.02.027

CuO thin films for the detection of H2S doses: Investigation and application: CuO thin films for the detection of H2S doses
Jörg Hennemann · Claus-Dieter Kohl · Bernd M. Smarsly · Tilman Sauerwald · Jean-Mathieu Teissier · Stefanie Russ · Thorsten Wagner
Physica Status Solidi (A) Applications and Materials 04/2015; 212(6):1281. DOI: 10.1002/pssa.201431735

Synthesis and morphological characterization of phenyl-modified macroporous–mesoporous hybrid silica monoliths
Rafael Meinusch · Kristof Hormann · Romana Hakim · Ulrich Tallarek · Bernd M. Smarsly
RSC Advances 02/2015; 5(26). DOI: 10.1039/C4RA16519E

Copper Oxide Based H2S Dosimeters–Modeling of Percolation and Diffusion Processes
Jörg Hennemann · Claus-Dieter Kohl · Bernd M. Smarsly · Hauke Metelmann · Marcus Rohnke · Jürgen Janek · Daniel Reppin · Bruno K. Meyer · Stefanie Russ · Thorsten Wagner
Sensors and Actuators B Chemical 02/2015; 217:41-50. DOI: 10.1016/j.snb.2015.02.001

Synthesis of silicon dioxide, silicon, and silicon carbide mesoporous spheres from polystyrene sphere templates
Lauren S. White · Julia Migenda · Xiaonan Gao · Dustin M. Clifford · Massimo F. Bertino · Khaled Mohammad Saoud · Christoph Weidmann · Bernd M. Smarsly
Journal of Sol-Gel Science and Technology 02/2015; DOI: 10.1007/s10971-015-3636-1

Morphological Analysis of Physically Reconstructed Silica Monoliths with Submicron Macropores: Effect of Decreasing Domain Size on Structural Homogeneity
Daniela Stoeckel · Christian Kübel · Marc O. Loeh · Bernd Michael Smarsly · Ulrich Tallarek
Langmuir 02/2015; 31(26). DOI: 10.1021/la5046018

Preparation and characterization of model catalysts for the HCl oxidation reaction
C. Kanzler · H. Over · B.M. Smarsly · C. Wessel
RSC Catalysis Series 01/2015; 2015(22):198-224.

Investigation of the Microstructure of Disordered, Non-­graphitic Carbons by an Advanced Analysis Method for Wide-Angle X-ray Scattering
Kristin Faber · Felix Badaczewski · Wilhelm Ruland · Bernd M. Smarsly
Zeitschrift für anorganische Chemie 12/2014; 640(15). DOI: 10.1002/zaac.201400210

From Macropores to Mesopores: 3D Morphology of Hierarchical Porous Solids
K. Hormann · D. Stoeckel · C. Kübel · A. Höltzel · B.M. Smarsly · U. Tallarek
Chemie Ingenieur Technik; 09/2014; DOI: 10.1002/cite.201450624

In-Depth Investigation of the Carbon Microstructure of Silicon Carbide-Derived Carbons by Wide-Angle X-ray Scattering
Kristin Faber · Felix Badaczewski · Martin Oschatz · Giovanni Mondin · Winfried Nickel · Stefan Kaskel · Bernd M. Smarsly
The Journal of Physical Chemistry C 07/2014; 118(29):15705-15715. DOI: 10.1021/jp502832x

Morphological Analysis of Disordered Macro-Mesoporous Solids Based on Physical Reconstruction by Nanoscale Tomography
Daniela Stoeckel · Christian Kübel · Kristof Hormann · Alexandra Hoeltzel · Bernd Michael Smarsly · Ulrich Tallarek
Langmuir 07/2014; 30(30). DOI: 10.1021/la502381m

Direct synthesis of carbide-derived carbon monoliths with hierarchical pore design by hard-templating
Winfried Nickel · Martin Oschatz · Martin von der Lehr · Matthias Leistner · Guang-Ping Hao · Philipp Adelhelm · Philipp Müller · Bernd M. Smarsly · Stefan Kaskel
07/2014; 2(32). DOI: 10.1039/C4TA02260B

Limits of ZnO Electrodeposition in Mesoporous Tin Doped Indium Oxide Films in View of Application in Dye-Sensitized Solar Cells
Christian Dunkel · Till von Graberg · Bernd M. Smarsly · Torsten Oekermann · Michael Wark
Materials 04/2014; 7:3291-3304. DOI: 10.3390/ma7043291

aktuelle Publikationen 2013/2014


An All Low-Temperature Fabrication of Macroporous, Electrochemically Addressable Anatase Thin Films
Schröder, M.; Sallard, S.; Böhm, M.; Einert, M.; Suchomski, C.; Smarsly, B. M.,; Mutisya, S.; Bertino, M.F.; Small, 2014, 10 (8): 1566-1574: DOI: 10.1002/smll.201300970

Coherent analysis of disordered mesoporous adsorbents using small angle X-ray scattering and physisorption experiments
Stöckel, D.; Wallacher, D.; Zichler, G.A.; Perlich, J.; Tallarek, U.; Smarsly, B. M.;Phys. Chem. Chem. Phys., 2014,16, 6583-6592,

DOI: 10.1039/C3CP55072A

Stable and Active Mixed Zr-Ce Oxides for Catalyzing the Tas Phase Oxidation of HCl
Urban, C.; Tarabanko, N.; Kanzler, C.H.; Zalewska-Wierzbicka, K.; Ellinghaus, R.; Rohrlack, S.F.; Chen, L.: Klar, P.J.; Smarsly, B.M.; Over, H.; Catalysis letters, 2013, 143 (12): 1362-1367,

DOI: 10.1007/s10562-013-1091-6

Hierarchically Ordered Monolithic Silica with Bimodal Porosity Obtained by Hydrolysis and Condensation of 1,4-Bis(trimethoxysilyl)arenes
von der Lehr,  M.; Weidmann, C.; Mascotto, S; Smarsly, B. M.; Chem-Ing-Tech 2013, 85 (11): 1700-1706

DOI: 10.1002/cite.201300079

Electrodeposition of zinc oxide on transparent conducting metal oxide nanofibers and its performance in dye sensitized solar cells
Dunkel, C.; Wark, M.; Oekermann, T.; Ostermann, R.; Smarsly, B. M.; Electrochim Acta 2013, 90: 375-381

DOI: 10.1016/j.electacat.2012.12.048

Electrospun Metal Oxide Nanofibres for the Assessment of Catalyst Morphological Stability under Harsh Reaction Conditions
Kanzler, C.H.; Urban, S.; Zalewska-Wierzbicka, K.; Hess, F.; Rohrlack, S.F.; Wessel, C.; Ostermann, R.; Hofmann, J.P.; Smarsly, B.M.; ChemCatChem 2013,

DOI: 10.1002/cctc.201300301

Bimodal Mesoporous Titanium Dioxide Anatase Films Templated by a Block Polymer and an Ionic Liquid: Influence of the Porosity on the Permeability
Sallard, Sébastien; Schröder, Michael; Boissière Cédric; Dunkel, Christian; Etienne, Mathieu; Walcarius, Alain; Oekermann, Torsten; Wark, Michael; Smarsly, B. M.; Nanoscale 2013, 5, 12316.

DOI: 10.1039/C3NR02732E